Be disorganized or messy. Virgos are very organized and efficient, so they may get frustrated if they perceive you as being disorganized or messy.
Be late or unreliable. Virgos value punctuality and reliability, so being late or unreliable may make them angry.
Be disrespectful of his opinions or beliefs. Virgos are very opinionated and passionate about what they believe, so disrespectful of their opinions or beliefs will likely make them angry.
Cheat on him or be unfaithful. Virgos are very loyal and faithful partners, so cheating on them or being unfaithful will likely devastate them and make them very angry.